TY - JOUR
T1 - Mesocosm constructed wetlands to remove micropollutants from wastewater treatment plant effluent
T2 - Effect of matrices and pre-treatments
AU - Lei, Yu
AU - Rijnaarts, Huub
AU - Langenhoff, Alette
PY - 2022/10
Y1 - 2022/10
N2 - The contamination of the aquatic environment by micropollutants (MPs) brings risks for the ecosystem and human health. Constructed wetlands (CWs) were an eco-friendly technology to remove MPs from wastewater treatment plant effluent. In this study, the removal of MPs was evaluated in seven vertical flow mesocosm CWs with different configurations, including different support matrices (sand and a combination of bark-biochar), light pre-treatments (UVC and sunlight) or bioaugmentation in support matrices (activated sludge). The CWs with bark-biochar as support matrix significantly enhanced the removal of irbesartan and carbamazepine (>40 %), compared to the CW filled with the conventional support matrix sand. UVC irradiation as pre-treatment was more efficient in removing MPs than sunlight irradiation. After UVC pre-treatment, less MPs accumulated in the plants in the subsequent CW unit compared to the CW unit without any pre-treatment. Moreover, in the UVC combined CW system, less sulfamethoxazole, furosemide, mecoprop and diclofenac were accumulated in the plants (<0.5 μg) than other MPs (>3 μg). The addition of 0.5 % activated sludge combined with the aeration of influent did not improve MP removal in the CW. Considering the application, a bark-biochar based CW combined with UVC pre-treatment will result in more MP removal than a conventional sand CW.
AB - The contamination of the aquatic environment by micropollutants (MPs) brings risks for the ecosystem and human health. Constructed wetlands (CWs) were an eco-friendly technology to remove MPs from wastewater treatment plant effluent. In this study, the removal of MPs was evaluated in seven vertical flow mesocosm CWs with different configurations, including different support matrices (sand and a combination of bark-biochar), light pre-treatments (UVC and sunlight) or bioaugmentation in support matrices (activated sludge). The CWs with bark-biochar as support matrix significantly enhanced the removal of irbesartan and carbamazepine (>40 %), compared to the CW filled with the conventional support matrix sand. UVC irradiation as pre-treatment was more efficient in removing MPs than sunlight irradiation. After UVC pre-treatment, less MPs accumulated in the plants in the subsequent CW unit compared to the CW unit without any pre-treatment. Moreover, in the UVC combined CW system, less sulfamethoxazole, furosemide, mecoprop and diclofenac were accumulated in the plants (<0.5 μg) than other MPs (>3 μg). The addition of 0.5 % activated sludge combined with the aeration of influent did not improve MP removal in the CW. Considering the application, a bark-biochar based CW combined with UVC pre-treatment will result in more MP removal than a conventional sand CW.
KW - Activated sludge
KW - Bark-biochar
KW - Constructed wetlands
KW - Micropollutants
KW - Sunlight
KW - UVC
U2 - 10.1016/j.chemosphere.2022.135306
DO - 10.1016/j.chemosphere.2022.135306
M3 - Article
C2 - 35714955
AN - SCOPUS:85132521001
SN - 0045-6535
VL - 305
JO - Chemosphere
JF - Chemosphere
M1 - 135306
ER -